I think that everything that's in print is available on the web site, but there are also web-only things, so the print magazine may be a bit of a "quality/triviality filter" in that regard.

I like The Atlantic in general, although I think they have a bit of what I sometimes call a "contrarian bias", e.g., prioritizing "the conventional wisdom is X, but here's why it's wrong" think-pieces even when their theses aren't particularly strong. (Slate and Salon were much worse about that in their heyday.)